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Compared with the gels sensitive to such stimuli as pH and heat, the studies on the light-responsive gels develop much more slowly There have been few reports concerning the photoinduced changes in shape or volume of the polymer gels for about 30 years, except that Irie and Suzuki et al have respectively done some excellent work on modi cation of the side chains of the gel networks with functional groups other than azobenzenes that either undergo ionization upon irradiation of UV light (Irie and Kungwatchakun, 1995; Ishikawa et al, 1991; Mamada et al, 1990; Irie, 1986) or cause local heating by absorbing energy from visible light (Suzuki et al, 1996; Suzuki and Tanaka, 1990) Recently, a successful strategy to manipulate the swelling response by light has been reported on poly(N-isopropylacrylamide) gels wherein the cross-links contain azobenzene groups.

Simple enough. Now do something useful with it, like doing a shortcode for promoting your RSS feed. 4. Starting with the function, this time you ll use it to output some HTML code as well, which gives you control of how the promotion appears:

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During the deswelling, irradiation of the gels with UV light was found to increase the expulsion of water from the swollen gels and decrease the water content of the gels by as much as 20% 30% They suggested that trans cis isomerization of the cross-links causes a local stress eld and lower entropy of the network, which in turn leads to an increase in unfavorable interaction of the network with the solvent, contributing to the increased expulsion of water from the gels Furthermore, an increase in the cross-link density was found to reduce the magnitude of this change (Mun-Sik and Vinay, 2002) Recently, semirigid poly(amide acid) gels containing azobenzene groups in the backbone structure were synthesized with a symmetric trifunctional cross-linker, 1,3,5-tris(4-aminophenyl) benzene (TAPB) (Fig 32).

function rss_promotion() { return '<div class="rsspromot">Never miss a beat - <a href="http://notesblog.com/feed/"> subscribe to the RSS feed!</a></div>'; }

Irradiation of laser light with the wavelength of 405 nm induced a local volume change in the gels owing to the deformation of the network structure, and the volume change was reversible by irradiation with visible light or heat The viscoelastic properties of the gels before and after light irradiation were also investigated, and a twofold increase in the storage modulus of the gels was observed upon irradiation of 405-nm laser light (Hosono et al, 2007)..

Figure 3.2. Synthesis route of poly(amide acid) gels containing azobenzene groups in their backbones and cross-linked with TAPB. Source: Hosono et al., 2007.

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to it:

Seki and coworkers (2007) developed a new type of photoresponsive polymer gel by introducing an azobenzene moiety on the mobile cyclodextrin part as the sliding cross-linking unit. The synthesis scheme of the gel is shown in Fig. 3.3. The polyrotaxane (PR) was composed of a noncovalent complex between poly(ethylene oxide) and a-cyclodextrin (a-CD, lling ratio: 28% of full complexation) capped with an adamantanamine unit at each end. Onto the sliding ring of CD, three types of azobenzene derivatives (6Az10-, 6Az(EO)3-, and CNAz(EO)3-) were linked by esteri cation. Gelation reactions, namely, formation of gure-of-eight sliding cross-linkages of the azobenzene-linked PR, were performed with 1,1carbonyl diimidazole in dimethyl-sulfoxide (DMSO). Figure 3.4 indicates volume changes of the gels in DMSO upon irradiation of alternate UV and visible light. For all three systems, irradiation of UV light induced expansion of the gels, and visible light the reverse. The change in D/D0 for 6Az10-PR gel reached 25%, which corresponds to a volume change of 80% 100%. It is inferred that such an effective molecule-to-material transformation can be ascribed to the dynamic nature of the cross-linkers (Sakai et al., 2007).

CH3(CH2)5

add_shortcode('rsspromo', 'rss_promotion');

6Az(EO)3

rss_promotion() function. All you have to do to wrap this up is to add some styling to the style.css stylesheet. Maybe something like this:

CNAz(EO)3

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